Extending the theory of lower bounds to reliability based on splits given by Guttman (1945), this paper introduces quantile lower bound coefficients λ4(Q ) that refer to cumulative proportions of potential “split-half” coefficients that are below a particular point Q in the distribution of split-halves based on different partitions of variables into two sets. Interesting quantile values are Q=.05,.50,.95,1.00 with λ4(.05)≤λ4(.50)≤λ4(.95)≤λ4(1.0) . Only λ4(1.0), Guttman’s maximal λ4, has previously been considered to be interesting, but in small samples it substantially overestimates population reliability ρ. The three coefficients λ4(.05), λ4(.50), and λ4(.95) provide new lower bounds to reliability. The smallest, λ4(.05), provides the most protection against capitalizing on chance associations and thus overestimation, λ4(.50) approximates coefficient α when α is an appropriate estimator of population reliability but improves on α otherwise, while λ4(.95) tends to overestimate reliability but also exhibits less bias than previous estimators. Computational theory, algorithm, and publicly available code based in R are provided to compute these coefficients. Simulation studies evaluate the performance of these coefficients and compare them to coefficient alpha and the greatest lower bound under several population reliability structures.